Cardcaptors, no.
As for CCS, there are two box sets: one has the first season, and the other has the second and third seasons. I got the series as the box sets, and they're pretty neat-looking. The first set looks like the Clow Book (the DVDs are on the "pages", and the episode list is on the inside cover), and the second looks like the Sakura Book. I got them a year ago, though, and you might have trouble finding them for a good price.
However, the moveis aren't in the box sets; you'll have to buy those separately. They're much easier to find, though.
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