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Haibane Renmei.
It's relaxing, tearjerking, and uplifting, and in that order. Easily the most beautiful and touching series I've ever seen.

Scrapped Princess had quite a few good tear jerkers too, as I recall.

Rozen Maiden was mostly happy, but had a handful of really powerful moments to its name.

There's also Someday's Dreamers -- I note that someone has already recommended its sequel.
AIR
HANDS FREAKING DOWN
YOU WILL CRY AT THE END!



Oh and FMA also has really sad moments, like the episode where that little girl and her dog became a chimera...
I was crying for like, a hour straight
got one dat one with zero and c2 w/e it was called brought a tear to my eye wait i think that was the one damn i forgot wait wait hold on hold on its ........ Death Note

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